OnCheckedChanged event not firing
Try turning AutoPostBack on for the checkbox control.
<asp:CheckBox ID="CheckBoxProcess" runat="server" Enabled="true" OnCheckedChanged = "CheckBoxProcess_OnCheckedChanged" AutoPostBack="true" />
This maybe the reason your method isn't being called.
Please try to check the value with the DB:
Checked='<%# Convert.ToBoolean(Eval("Processed"))
%>'